As I said in my comment, one of your declarations is wrong and because of that, the unexpected result. Please, try understanding the next (didactic) code, to clarify the issue:
Sub testArray1D2D()
Dim arr1D, arr2DStrange, arr2D, i As Long
arr1D = Split("a,b,c,d,e,f,g,h,i,j", ",")
ReDim arr2DStrange(10, 1): ReDim arr2D(1 To 10, 1 To 1)
For i = 0 To UBound(arr1D)
arr2DStrange(i, 1) = arr1D(i)
arr2D(i + 1, 1) = arr1D(i)
Next i
Range("A2").Resize(UBound(arr2DStrange), 1).value = arr2DStrange 'it returns nothing
Range("B2").Resize(UBound(arr2DStrange), 2).value = arr2DStrange 'it returns what you need in the second column (D:D)
Range("D2").Resize(UBound(arr2D), 1).value = arr2D 'it returns correctly (what you need)
Range("E2").Resize(UBound(arr1D) + 1, 1).value = Application.Transpose(arr1D) 'also correct (a 1D array does not have any column! and it must be transposed. Otherwise, it repeats its first element value)
End Sub
When use declaration Dim test22(10, 1) As Integer it creates a 2D array but it has two columns. It is the equivalent of Dim test22(0 to 10, 0 to 1) As Integer. When you fill only the second column (1) and try returning the first one (0), this column, is empty.
The correct declaration for obtaining a 2D array with 10 rows and 1 column should be Dim test22(1 to 10, 1 to 1) As Integer.
Then, iTemp = CInt(UBound(dat1)) declares a 1D array of 11 elements (from 0, inclusive, to 10). And you never loaded its first element, starting iteration with 1. That's why the line Sheets("Info").Range("G1:G10").Value2 = NumMatches returned the first empty element 10 times... If your code would fill correctly the first element and if it was a matching one, your code will return 10 rows of 1 value.
NumMatches(iCompareOuter) = NumMatches(iCompareOuter) + 1 is the equivalent of NumMatches(iCompareOuter) = 1. NumMatches(iCompareOuter) is always empty in that moment...
And it is good to cultivate the habit to avoid declarations As Integer in such a case. Working with Excel rows, the value of an Integer must be exceeded. Try using As Long. VBA is so designed to make the memory working in the same way, without any supplementary stress.
A more compact way to accomplish what you need will be the next approach:
Sub Comparor()
Dim dat1(), dat2(), NumMatches(), mtch, i As Long
dat1() = Sheets("Data1").Range("E1:E10").Value2
dat2() = Sheets("Data2").Range("E1:E10").Value2
ReDim NumMatches(1 To UBound(dat1), 1 To 1)
For i = 1 To UBound(dat1)
mtch = Application.match(dat1(i, 1), dat2, 0)
If IsNumeric(mtch) Then NumMatches(i, 1) = "OK"
Next i
Sheets("Info").Range("G1:G10").Value2 = NumMatches
End Sub
Not tested, but it should work. Except the case of a typo, when an error will be raised and sending some feedback I will rapidly correct...