The request failed with HTTP status 401: Unauthorized

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I have a .NET 2.0 website (VB) running in my IIS6 (XP Pro SP2) and a .NET 3.5 (configured as .NET2 under IIS's ASP.NET tab, of course) hosting an ASMX web service.

In Chrome, I can call the ASMX and invoke the web methods successfully. However, in calling the web methods in code, from the .NET 2.0 website I get:

The request failed with HTTP status 401: Unauthorized.

How do I get around this?

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